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In addition to the aforementioned reasons, the following two reasons are included as possible factors that cause the crack to move more slowly in PFS than in NPS, considering that the crack moves through the matrix material. The first reason is the presence of pores that are smaller than the size of the matrix material. As can be seen in Fig. 5(a)-5(d), the region of the matrix material is covered by the pores. Furthermore, the pores are connected to each other via thin films (interfacial crack surfaces), which are responsible for crack propagation. We consider that these interfacial crack surfaces and pores contribute to slow crack propagation in PFS. The second reason is the presence of lower toughness of PFS, which leads to large size of the yielding zone as well as a crack-free zone. These two aspects contribute to slow crack propagation in PFS. On the other hand, in NPS, the region of the matrix material is not covered by pores; therefore, the presence of pores is less relevant for the present results on crack propagation. The toughness of PFS is lower than that of NPS, which is one of the reasons why the crack tends to propagate in PFS much more slowly.
By using the present polymer sheets, we first investigate whether the sizes of the representative structural size play a significant role in crack propagation. Besides the size of pore, we also vary the size of matrix materials to assess the effect of the representative structural size on crack propagation. Based on the obtained results, we discuss the fracture behavior of both PFS and NPS. In the present study, a crack propagates through the matrix material in a laminar mode, with the crack being straight and parallel to the boundary of the matrix material (the boundary in the x-y plane). This is similar to a straight crack in non-porous polymer materials.
It is interesting that the present results show that the crack velocity in PFS and NPS behave differently, even though they have similar bulk viscoelastic properties. It would be helpful to understand why the results observed here are so different from those reported in the literature. In the present study, the films were prepared in polymer sheets with the same pore size (20 μm); however, the size of the pore was much larger for PFS (300 μm) than for NPS (20 μm).
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